Sorry, no online dictionaries contain the exact phrase unnatural grimace.
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Reverse dictionary results:
1. mak
2. make
3. pallor
4. ruddy
5. act
6. deform
7. bord
8. color
9. complexion
10. dimpled
11. facade
12. false face
13. forehead
14. gargoyle
15. gurn
16. manducus
17. mascaron
18. mask
19. masking
20. paint
21. tight
22. lividity
23. face
24. leer
25. mouth
26. mouthing
27. smirk
28. odor
29. pull
30. react
31. abandon
32. account
33. acromegaly
34. address
35. afford
36. aim
37. air
38. aloe
39. answer
40. answering

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You can look up the words in the phrase individually using these links:   unnatural ?   grimace ?
(A question mark next to a word above means that we couldn't find it, but clicking the word might provide spelling suggestions.)

Not helpful? You might try using the wildcards * and ? to find the word you're looking for. For example, use
unna*to search for words beginning with unna, or
*maceto search for words ending with mace
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