Sorry, no online dictionaries contain the exact phrase the most important thing.
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Reverse dictionary results:
1. priority
2. paramountcy
3. significance
4. essence
5. centrality
6. consignificative
7. being
8. essent
9. formally
10. originative
11. particularism
12. significatory
13. substantive
14. cardinally
15. causer
16. companionably
17. consignificant
18. consubstantiate
19. correctively
20. dasein
21. democratically
22. educationally
23. entrepreneurially
24. personably
25. personalism
26. prescriptively
27. rule
28. significancy
29. standard
30. statutorily
31. subsistential
32. that
33. canonical
34. causation
35. cause
36. complicitly
37. conventionally
38. essential
39. executively
40. formal

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You can look up the words in the phrase individually using these links:   the ?   most ?   important ?   thing ?
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