Sorry, no online dictionaries contain the exact phrase the most important.
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Reverse dictionary results:
1. crucial
 2. paramount
3. essential
4. vital
5. significant
6. central
7. consequential
8. imperative
9. instrumental
10. key
 11. of the essence
12. pivotal
13. cardinal
14. mission-critical
15. predominantly
16. predominately
17. prevalently
18. relevant
19. significative
20. substantial
 21. built-in
22. capitally
23. constitutive
24. core
25. cruciality
26. first
27. majorly
28. material
29. meaningful
30. powerful
 31. predominant
32. summum bonum
33. all-important
34. being
35. by and large
36. coessential

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