Sorry, no online dictionaries contain the exact phrase most important thing.
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Reverse dictionary results:
1. crucial
 2. essential
3. primary
4. significant
5. paramount
6. built-in
7. core
8. imperative
9. main
10. main thing
 11. mission-critical
12. maine
13. of the essence
14. vital
15. basic
16. central
17. chiefly
18. coessential
19. constitutive
20. first and foremost
 21. instrumental
22. mainprize
23. prevalently
24. prime
25. behavior
26. capitall
27. cardinal
28. dominate
29. in general
30. key
 31. mostly
32. name of the game
33. predominately
34. primacy effect
35. primarily

You can look up the words in the phrase individually using these links:   most ?   important ?   thing ?
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